Notes

Surfactant-free synthesis involving covalent natural construction nanospheres within water from 70 degrees.
Inspired by the idea of non-Hermitian spectral engineering and non-Hermitian skin effect, a novel, to the best of our knowledge, design for stable emission of coupled laser arrays with tunable phase locking and strong supermode competition suppression is suggested. We consider a linear array of coupled resonators with asymmetric mode coupling displaying the non-Hermitian skin effect and show that, under suitable tailoring of complex frequencies of the two edge resonators, the laser array can stably emit in a single extended supermode with tunable phase locking and with strong suppression of all other skin supermodes. The proposed laser array design offers strong robustness against both structural imperfections of the system and dynamical instabilities typical of semiconductor laser arrays.We have developed a bidirectional focusing microscope that utilizes feedback-assisted wavefront shaping to focus light inside a heterogenous material in order to monitor sub-surface chemical reactions. The bidirectional geometry is found to provide superior intensity enhancement relative to single-sided focusing, owing to increased mode control and long-range mesoscopic correlations. Also, we demonstrate the microscope's capability to measure sub-surface chemical reactions by optically monitoring the photodegradation of a Eu-doped organic molecular crystal embedded in a heterogeneous material using both fluorescence and Raman spectroscopy as probe techniques.A kind of plasmonic nanostructure is proposed that can generate the arbitrary superposition of orbital angular momentum (OAM) states in surface plasmons (SPs), which is achieved by combining the segmented spirals with nanoslit pairs. The structures can independently modulate both the phase and amplitude of SP waves, and thus enable the superposition of two OAM states with arbitrary topological charges (TCs) as well as free control of their relative amplitudes. Superposed states distributed over the entire Bloch sphere and hybrid superposed states with different TCs were constructed and experimentally demonstrated. This work will offer more opportunities for multifunctional plasmonic devices.Surface-enhanced Raman scattering (SERS) spectroscopy has attracted tremendous interest as a highly sensitive label-free tool to detect pollutants in aqueous environments. However, the high cost and poor reusability of conventional SERS substrates restrict their further applications in rapid and reproducible pollutant detection. Here, we report a reliable optical manipulation method to achieve rapid photothermal self-assembly of Au nanoparticles (AuNPs) in water within 30 s by a tapered optical fiber, which is utilized for highly sensitive SERS substrate preparation. The results show that the SERS substrate achieves low detection limits of 10-9 mol/L with an enhancement factor (EF) of 106 for chemical pollutants solutions, including thiram, pyrene, and rhodamine 6G. The SERS enhancement effect based on assembled AuNPs was more than 20 times that based on a gold colloid solution. As a result, the smart reversible assembly of AuNPs exhibits switchable plasmonic coupling for tuning SERS activity, which is promising for the application of SERS-based sensors and environmental pollutant detection.We present an artificial birefringent space-variant polarization converter for the near infrared, λ = 1550 nm. Each hollow waveguide has a rectangular shape with lateral dimensions of 1550 nm in the x-direction and 1034 nm as the largest length in the y-direction. The whole device consists of approximately 2000 × 2500 hollow waveguides realized in a 2-µm-thick gold structure. They are separated by sidewalls with a width of less than 500 nm. By proper choice of the lateral widths of the individual holes, a pixel-wise polarization conversion of an incoming wave field is possible. By suitable choice of the fabrication parameters, a birefringent phase shift up to 2π can be achieved. Hence, the structure is able to fully convert the state of polarization, e.g., from linear to circular. For fabrication of the device, femtosecond 3D direct laser writing was combined with electroplating. Here, we describe the operation of our device as a space-variant polarization converter by measuring the angle-dependent transmitted power and by calculating the ellipticity and the phase delay dependent on position as well as the azimuth angle from the experimentally determined powers.We analyze the lineshape of the extraordinary optical transmission (EOT) associated with surface plasma waves (SPWs) excited with a metal photonic crystal (MPC), an Au film perforated with a 2.6 µm period, two-dimensional array of holes, integrated atop a GaAs substrate. From its asymmetry by Fano interference between transmission mediated by SPWs and direct transmission through individual holes, the resonance energy of the fundamental SPW propagating along the MPC/GaAs interface is extracted as 138.8 meV. This energy, the reference of the analysis, is slightly higher than the energy of the apparent peak of the EOT but lower than that of the Rayleigh anomaly closely related to the direct transmission. Its accuracy is verified with an identical MPC integrated on a quantum dot infrared photodetector coupled to the same SPW. Additional lineshape parameters, including relative strength of the two pathways to the transmission and SPW broadening, are determined from experiments. A condition of the Fano interference for EOT, critical to the intensity of its peak transmission, is established with their relations.An integrated sampled-grating silicon hybrid mode-locked ring laser is proposed for 20-GHz super-mode noise suppression. The dynamics, phase noise, and timing jitter are investigated using a delay differential equation (DDE) model. The results show that the 20-GHz harmonic regime of the proposed structure is significantly increased when the sampled-grating structure is included. Additionally, a better selectivity of the optical modes by a sampled-grating distributed Bragg reflector (SGDBR) leads to more suppression of super-mode noise compared to the long-ring structures with a spectral filter which were previously reported. Compared to previous works, the phase noise is improved by approximately 6 dB and the timing jitter is decreased to less than a third.We consider the spectral-domain counterparts of spatial-domain polarization gratings and study their effect on the temporal evolution of femtosecond-scale light pulses. These devices divide an incident light pulse to several orders via spectral polarization modulation, permitting pulse splitting and shaping with controlled time-domain polarization dynamics.Reinforcement learning (RL) is applied to improve the performance of the polarization modulator (PolM)-based W-band radio-over-fiber (RoF) system in this Letter. By controlling the polarization angle of the dual-wavelength laser source in the PolM-based scheme, the RF response can be easily modified and therefore it hugely increases the available bandwidth in the RoF system. In the proposed RL scheme, the state is described as the value of the angle from the polarization controller (PC). We use changing the angle of the polarizer (P) as the actions of the RL agent to optimize the frequency response. The agent also receives a reward from the system and learns from the environment and previous experience. Moreover, the reward is the value of error vector magnitude at each state. Therefore, the proposed scheme of RL is implemented and demonstrated in a multi-channel RoF system, and the results show that an RL agent provides an effective intelligent technique to obtain the best quality of data transmission.A fully integrated waveguide-based, efficient surface plasmon coupler composed of a realistic non-tapered dielectric waveguide with graphene patches and sheet is designed and optimized for the infrared. The coupling efficiency can reach nearly 80% for a coupler as short as 700 nm for an operating wavelength of 12 μm. This work is carried out using rigorous numerical models based on the finite element method taking into account 2D materials as surface conductivities. The key numerical results are supported by physical arguments based on modal approach or resonance condition.A computationally efficient radiative transport model is presented that predicts a camera measurement and accounts for the light reflected and blocked by an object in a scattering medium. The model is in good agreement with experimental data acquired at the Sandia National Laboratory Fog Chamber Facility (SNLFC). The model is applicable in computational imaging to detect, localize, and image objects hidden in scattering media. Here, a statistical approach was implemented to study object detection limits in fog.Integrated optical phased array (OPA) devices have been widely studied as a solution for solid-state light detection and ranging technology in the autonomous driving application. https://www.selleckchem.com/products/pf-07265807.html In this work, a phase-combining unit (PCU) is proposed and studied. With a given number (N) of phase shifters, instead of the general N (phase shifters) to N (emitters) control, the PCU can enable an N to 2N-1 control, which efficiently suppresses the aliasing effect. The theoretical analysis, numerical simulation, and experimental proof-of-concept have been completed in this work. The results show that a maximum suppression of 92.54% can be achieved for the grating lobes in simulation, and an average 53.76% is tested for one grating lobe in the experiment. In conclusion, the PCU can be used as a universal aliasing suppression unit on many types of integrated OPA devices.All-dielectric nanophotonics offers a wide range of possibilities for thermally induced light manipulation at the nanoscale. High quality resonances allow for efficient light-to-heat conversion supported by various temperature detection approaches based on thermally sensitive intrinsic optical responses. In this work, we study theoretically a phenomenon of the photothermal reshaping of the radiation pattern of second-harmonic generation (SHG) that occurs in resonant all-dielectric systems. In the suggested geometry, a near-IR pulsed laser is used for SHG while a continuous wave visible laser simultaneously heats the structure. The thermo-optical switching of the resonant optical states in the nanostructures governs the reconfiguration of the emission pattern, without significant loss in the magnitude of the SHG. We believe, that our findings will pave the way for subwavelength-size near-IR thermally switchable nonlinear optical devices.The ability of hemodilution to improve vascular circulatory impairment has been demonstrated. However, the effects of acute hemodilution on cerebral hemodynamics and oxygen metabolism have not been assessed at the microscopic level, due to technical limitations. To fill this void, we have developed a new, to the best of our knowledge, photoacoustic microscopy system, which enables high-speed imaging of blood hemoglobin concentration, oxygenation, flow, and oxygen metabolism in vivo. The system performance was examined in both phantoms and the awake mouse brain. This new technique enabled wide-field (4.5 × 3 mm2) multi-parametric imaging of the mouse cortex at 1 frame/min. Narrowing the field of view to 1.5 × 1.5 mm2 allowed dynamic imaging of the cerebral hemodynamic and metabolic responses to acute hypervolemic hemodilution at 6 frames/min. Quantitative analysis of the hemodilution-induced cerebrovascular responses over time showed rapid increases in the vessel diameter (within 50-210 s) and blood flow (50-210 s), as well as decreases in the hemoglobin concentration (10-480 s) and metabolic rate of oxygen (20-480 s) after the acute hemodilution, followed by a gradual recovery to the baseline levels in 1440 s.
Read More: https://www.selleckchem.com/products/pf-07265807.html