Notes

Intonation associated with Visual Phonons within α-MoO3-VO2 Multilayers.
We demonstrate a methodology for predicting particle removal efficiency of polypropylene-based filters used in personal protective equipment, based on quantification of disorder in the context of methyl group orientation as structural motifs in conjunction with an Ising model. The corresponding Bragg-Williams order parameter is extracted through either Raman spectro-scopy or scanning electron microscopy. Temperature-dependent analysis verifies the presence of an order-disorder transition, and the methodology is applied to published data for multiple samples. SB203580 The result is a method for predicting the particle removal efficiency of filters used in masks based on a material-level property.Water scarcity is one of the greatest global challenges at this time. Significant efforts have been made to harvest water from the air, due to widely available water sources present in the atmosphere. Particularly, solar-driven hygroscopic water harvesting based on the adsorption-desorption process has gained tremendous attention because of the abundance of solar energy in combination with substantial improvements in conversion efficiency enabled by advanced sorbents, improved photothermal materials, interfacial heating system designs, and thermal management in recent years. Here, recent developments in atmospheric water harvesting are discussed, with a focus on solar-driven hygroscopic water harvesting. The diverse structural designs and engineering strategies that are being used to improve the rate of the water production, including the design principles for sorbents with high adsorption capacity, high-efficiency light-to-heat conversion, optimization of thermal management, vapor condensation, and water collection, are also explored. The current challenges and future research opportunities are also discussed, providing a roadmap for the future development of solar-driven hygroscopic water harvesting technology.Solar-powered interfacial evaporation, a cost-effective and ecofriendly way to obtain freshwater from contaminated water, provides a promising path to ease the global water crisis. However, solute accumulation has severely impacted efficient light-to-heat-to-vapor generation in conventional solar evaporators. Here, it is demonstrated that an interfacial solar thermal photo-vapor generator is an efficient light-to-heat photo-vapor generator that can evaporate water stably in the presence of solute accumulation. An energy downconversion strategy which shifts sunlight energy from visible-near infrared to mid infrared-far infrared bands turns water from transparent to its own absorber, thus changing the fixed evaporation surface (black absorber) in a traditional solar evaporator to a dynamic front (solute surface). Light reflected from the solute can be recycled to drive evaporation. The prototype evaporator can evaporate at a high speed of 1.94 kg m-2 h-1 during a persistent solute accumulation process for 32 h. Such an ability to produce purified water while recycle valuable heavy metals from waste water containing heavy metal ions can inspire more advanced solar-driven water treatment devices.The solar-assisted desalination generator (SADG) shows great potential for solving water scarcity problems. However, salt precipitation and accumulation is still a challenge for SADG, which slows down solar steam generation performance of evaporator during operation. Here, a facile integrative evaporator featuring stable and high evaporation performance breaks this bottleneck. By using a rational design in which amorphous carbon particles are evenly composited within the porous chitosan aerogel, the evaporator not only integrates excellent light absorption, heat management, and water transportation abilities but also endows a large vapor escape space. Upon desalination, salt concentration ingredients between carbon particles and chitosan membranes can be quickly balanced by water transport in interconnected chitosan chains, and thus salt precipiation on the evaporator surface would be avoided. Compared to other salt-rejection evaporators, the integrative evaporator can operate in 3.5 wt% brine for 60 days without salt precipiation and exhibits a stable evaporation rate (1.70 kg m-2 h-1), indicating its potential for practical applications in seawater desalination and the harvest of clean drinking water.Renewable energy harvesting from the sun and outer space have aroused significant interest over the past decades due to their great potential in addressing the energy crisis. Furthermore, the harvested renewable energy has benefited another global challenge, water scarcity. Both solar steam generation and passive radiative cooling-enabled atmospheric water harvesting are promising technologies that produce freshwater in green and sustainable ways. Spectral control is extremely important to achieve high efficiency in the two complementary systems based on absorbing/emitting light in a specific wavelength range. For this reason, a broad variety of solar absorbers and IR emitters with great spectral selectivity have been developed. Although operating in different spectral regions, solar selective absorbers and IR selective emitters share similar design strategies. At this stage, it is urgent and necessary to review their progress and figure out their common optical characteristics. Herein, the fundamental mechanisms and recent progress in solar selective absorbers and IR selective emitters are summarized, and their applications in water production are reported. This review aims to identify the importance of selective absorbers/emitters and inspire more research works on selective absorbers/emitters through the summary of advances and the establishment of the connection between solar absorbers and IR emitters.Solar-powered water evaporation is a primitive technology but interest has revived in the last five years due to the use of nanoenabled photothermal absorbers. The cutting-edge nanoenabled photothermal materials can exploit a full spectrum of solar radiation with exceptionally high photothermal conversion efficiency. Additionally, photothermal design through heat management and the hierarchy of smooth water-flow channels have evolved in parallel. Indeed, the integration of all desirable functions into one photothermal layer remains an essential challenge for an effective yield of clean water in remote-sensing areas. Some nanoenabled photothermal prototypes equipped with unprecedented water evaporation rates have been reported recently for clean water production. Many barriers and difficulties remain, despite the latest scientific and practical implementation developments. This Review seeks to inspire nanoenvironmental research communities to drive onward toward real-time solar-driven clean water production.
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