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This shifts the FL closer to the Dirac point, allowing investigating the physics of the Dirac and Weyl points, making this compound a platform for the investigation of the Dirac and Weyl points in three-dimensional materials.Objective. The main objective of this study was to assess the feasibility of lowering the hardware requirements for fast neural electrical impedance tomography (EIT) in order to support the distribution of this technique. Specifically, the feasibility of replacing the commercial modules present in the existing high-end setup with compact and cheap customized circuitry was assessed.Approach. Nerve EIT imaging was performed on rat sciatic nerves with both our standard ScouseTom setup and a customized version in which commercial benchtop current sources were replaced by custom circuitry. Electrophysiological data and images collected in the same experimental conditions with the two setups were compared. Data from the customized setup was subject to a down-sampling analysis to simulate the use of a recording module with lower specifications.Main results. selleck Compound action potentials (573 ± 287μV and 487 ± 279μV,p=0.28) and impedance changes (36 ± 14μV and 31 ± 16μV,p=0.49) did not differ significantly when measured using commercial high-end current sources or our custom circuitry, respectively. Images reconstructed from both setups showed neglibile ( less then 1voxel, i.e. 40μm) difference in peak location and a high degree of correlation (R2 = 0.97). When down-sampling from 24 to 16 bits ADC resolution and from 100 to 50 KHz sampling frequency, signal-to-noise ratio showed acceptable decrease ( less then -20%), and no meaningful image quality loss was detected (peak location difference less then 1voxel, pixel-by-pixel correlationR2 = 0.99).Significance The technology developed for this study greatly reduces the cost and size of a fast neural EIT setup without impacting quality and thus promotes the adoption of this technique by the neuroscience research community.We report sensing of single nanoparticles using disordered metallic nanoisland substrates supporting surface plasmon polaritons (SPPs). Speckle patterns arising from leakage radiation of elastically scattered SPPs provide a unique fingerprint of the scattering microstructure at the sensor surface. Experimental measurements of the speckle decorrelation are presented and shown to enable detection of sorption of individual gold nanoparticles and polystyrene beads. Our approach is verified through bright-field and fluorescence imaging of particles adhering to the nanoisland substrate.Random nanowire networks (NWNs) are regarded as promising memristive materials for applications in information storage, selectors, and neuromorphic computing. The further insight to understand their resistive switching properties and conduction mechanisms is crucial to realize the full potential of random NWNs. Here, a novel planar memristive device based on necklace-like structure Ag@TiO2NWN is reported, in which a strategy only using water to tailor the TiO2shell on Ag core for necklace-like core-shell structure is developed to achieve uniform topology connectivity. With analyzing the influence of compliance current on resistive switching characteristics and further tracing evolution trends of resistance state during the repetitive switching cycles, two distinctive evolution trends of low resistance state failure and high resistance state failure are revealed, which bear resemblance to memory loss and consolidation in biological systems. The underlying conduction mechanisms are related to the modulation of the Ag accumulation dynamics inside the filaments at cross-point junctions within conductive paths of NWNs. An optimizing principle is then proposed to design reproducible and reliable threshold switching devices by tuning the NWN density and electrical stimulation. The optimized threshold switching devices have a high ON/OFF ratio of ∼107with threshold voltage as low as 0.35 V. This work will provide insights into engineering random NWNs for diverse functions by modulating external excitation and optimizing NWN parameters to satisfy specific applications, transforming from neuromorphic systems to threshold switching devices as selectors.Motivated by the recent successful synthesis of 2D quintuple-layer atomic materials, for the first time, we design and investigate the electronic and transport properties of Janus Al2XY2(X/Y = S, Se, Te; X ≠ Y) monolayers by using the density functional theory. Our calculations demonstrate that most of the models of Al2XY2(except for Al2STe2monolayer) are dynamically and mechanically stable. By using the hybrid functional, all models of Al2XY2are semiconductors with an indirect bandgap. Meanwhile, Al2TeS2monolayer is found to be metal at the Perdew-Burke-Ernzerhof level. Due to the vertical asymmetry structure, an intrinsic built-in electric field exists in the Al2XY2and leads to a difference in the vacuum levels between the two sides of the monolayers. Carrier mobilities of Al2XY2monolayers are high directional anisotropic due to the anisotropy of their deformation potential constant. Al2XY2monolayers exhibit high electron mobility, particularly, the electron mobility of Al2SeS2exceeds 1 × 104cm2V-1 s-1, suggesting that they are suitable for applications in nanometer-sized electronic devices.Magnetically actuated micro/nanorobots are typical micro- and nanoscale artificial devices with favorable attributes of quick response, remote and contactless control, harmless human-machine interaction and high economic efficiency. Under external magnetic actuation strategies, they are capable of achieving elaborate manipulation and navigation in extreme biomedical environments. This review focuses on state-of-the-art progresses in design strategies, fabrication techniques and applications of magnetically actuated micro/nanorobots. Firstly, recent advances of various robot designs, including helical robots, surface walkers, ciliary robots, scaffold robots and biohybrid robots, are discussed separately. Secondly, the main progresses of common fabrication techniques are respectively introduced, and application achievements on these robots in targeted drug delivery, minimally invasive surgery and cell manipulation are also presented. Finally, a short summary is made, and the current challenges and future work for magnetically actuated micro/nanorobots are discussed.Neural network quantum states provide a novel representation of the many-body states of interacting quantum systems and open up a promising route to solve frustrated quantum spin models that evade other numerical approaches. Yet its capacity to describe complex magnetic orders with large unit cells has not been demonstrated, and its performance in a rugged energy landscape has been questioned. Here we apply restricted Boltzmann machines (RBMs) and stochastic gradient descent to seek the ground states of a compass spin model on the honeycomb lattice, which unifies the Kitaev model, Ising model and the quantum 120° model with a single tuning parameter. We report calculation results on the variational energy, order parameters and correlation functions. The phase diagram obtained is in good agreement with the predictions of tensor network ansatz, demonstrating the capacity of RBMs in learning the ground states of frustrated quantum spin Hamiltonians. The limitations of the calculation are discussed. A few strategies are outlined to address some of the challenges in machine learning frustrated quantum magnets.Developing highly efficient and non-precious materials for Zn-air batteries (ZABs) and supercapacitors (SCs) are still crucial and challenging. Herein, electronic reconfiguration and introducing conductive carbon-based materials are simultaneously conducted to enhance the ZABs and SCs performance of Co2P. We develop a simple and efficient electrospinning technology followed by carbonization process to synthesize embedding Co2P nanoparticles in Cu doping carbon nanofibers (Cu-Co2P/CNFs). As a result, the 7% Cu-Co2P/CNFs presents high oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) activity (half-wave potential of 0.792 V for ORR, an overpotential of 360 mV for OER). The ZABs exhibit a power density of 230 mW cm-2and excellent discharge-charge stability of 80 h. In addition, the 7% Cu-Co2P/CNFs show the specific capacitance of 558 F g-1at 1 A g-1. Moreover, the 7% Cu-Co2P/CNFs//CNFs asymmetric supercapacitor was assembled applying 7% Cu-Co2P/CNFs electrode and pure CNFs, which exhibits a high energy density (25.9 Wh kg-1), exceptional power density (217.5 kW kg-1) and excellent cycle stability (96.6% retention after 10 000 cycles). This work may provide an effective way to prepared Co2P based materials for ZABs and SCs applications.Metal oxides are well-known materials that have been considered as the prominent photocatalysts. Photocatalysis is a promising way to address the environmental issues which are caused by fossil fuel the combustion and industrial pollutants. Lot of efforts such as doping of metal oxides with metals, non-metals have been made to enhance their photocatalytic activity. More specifically, in this review we have discussed detailed synthesis procedures of rare earth doped metal oxides performed in the past decades. The advantage of doping metal oxides with rare earth metals is that they readily combine with functional groups due to the 4f vacant orbitals. Moreover, doping rare earth metals causes absorbance shift to the visible region of the electromagnetic spectrum which results to show prominent photocatalysis in this region. The effect of rare earth doping on different parameters of metal oxides such as band gap and charge carrier recombination rate has been made in great details. In perspective section, we have given a brief description about how researchers can improve the photocatalytic efficiencies of different metal oxides in coming future. The strategies and outcomes outlined in this review are expected to stimulate the search for a whole new set of rare earth doped metal oxides for efficient photocatalytic applications.Objective. Lower limb amputees suffer from a variety of functional deficits related to the absence of sensory communication between the central nervous system and the lost extremity. Indeed, they experience high risk of falls, asymmetric walking and balance, and low prosthesis embodiment, that significantly decrease their quality of life. Presently, there are no commercially available devices able to provide sensory feedback to leg amputees but recently some invasive solutions (i.e. requiring surgery) have been proposed by different research groups. However, a non-invasive effective alternative exploitable in everyday life is still missing.Approach. To address this need we developed and tested a lightweight, non-invasive, wearable technology (NeuroLegs) providing sensory (i.e. knee angle joint and tactile) feedback to the users through electro-cutaneous stimulation. Standard mechanical and electrical tests were performed to assess the safety and reliability of the technology. The NeuroLegs system was verified that can be successfully exploited in different walking conditions of daily life.
My Website: https://www.selleckchem.com/products/bay-2666605.html
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